Continental rifting is an important geodynamic process during which the Earth's outer-most rigid shell undergoes continuous stretching resulting in continental break-up and theformation of new oceanic basins. The East African Rift System, which has two continentalsegments comprising largely of the East African Rift (EAR) to the West and the easternmostsegment Madagascar, is the largest narrow rift on Earth. However, the driving mechanismsof continental rifting remain poorly understood due to a lack of numerical infrastructure tosimulate rifting, the lack of knowledge of the underlying mantle dynamics, and poor knowl-edge of mantle rheology. Here, we use state-of-art computational modeling of the upper660 km of the Earth to: 1) provide a better understanding of mantle flow patterns and themantle rheology beneath Madagascar, 2) to elucidate the main driving forces of observedpresent-day∼E-W opening in the EAR, and 3) to investigate the role of multiple plumesor a superplume in driving surface deformation in the EAR. In chapter 1, we simulate EdgeDriven convection (EDC), constrained by a lithospheric thickness model beneath Madagas-car. The mantle flow associated with the EDC is used to calculate induced olivine aggregates'Lattice Preferred Orientation (LPO), known as seismic anisotropy. The predicted LPO isthen used to calculate synthetic seismic anisotropy, which were compared with observationsacross the island. Through a series of comparisons, we found that asthenospheric flow result-ing from undulations in lithospheric thickness variations is the dominant source of the seismicanisotropy, but fossilized structures from an ancient shear zone may play a role in southern

Madagascar. Our results suggest that the rheological conditions needed for the formationof seismic anisotropy, dislocation creep, dominates the upper asthenosphere beneath Mada-gascar and likely other continental regions. In chapter 2, we use a 3D numerical model ofthe lithosphere-asthenosphere system to simulate instantaneous lithospheric deformation inthe EAR and surroundings. We test the hypothesis that the∼E-W extension of the EAR isdriven by large scale forces arising from topography and internal density gradients, known aslithospheric buoyancy forces. We calculate surface deformation solely driven by lithosphericbuoyancy forces and compare them with surface velocity observations. The lithosphericbuoyancy forces are implemented by imposing observed topography at the model surfaceand lateral density variations in the crust and mantle down to a compensation depth of 100km. Our results indicate that the large-scale∼E-W extension across East Africa is driven bylithospheric buoyancy forces, but not along-rift surface motions in deforming zones. In chap-ter 3, we test the hypothesis that the anomalous northward rift-parallel deformation observedin the deforming zones of the EAR is driven by viscous coupling between the lithosphereand deep upwelling mantle material, known as a superplume, flowing northward. We testtwo end-member plume models including a multiple plumes model simulated using high res-olution shear wave tomography-derived thermal anomaly and a superplume model (Africansuperplume) simulated by imposing a northward mantle-wind on the multiple plumes model.Our results suggest that the horizontal tractions from northward mantle flow associated withthe African Superplume is needed to explain observations of rift-parallel surface motions indeforming zones from GNSS/GPS data and northward oriented seismic anisotropy beneaththe EAR. Overall, this work yields a better understanding of the geodynamics of Africa.