Browsing by Author "Kang, Han Byul"
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- High-Efficiency Skutterudite Modules at a Low Temperature GradientLi, Wenjie; Stokes, David; Poudel, Bed; Saparamadu, Udara; Nozariasbmarz, Amin; Kang, Han Byul; Priya, Shashank (MDPI, 2019-11-11)Thermoelectric skutterudite materials have been widely investigated for their potential application in mid-temperature waste heat recovery that has not been efficiently utilized A large amount of research has focused on developing materials with a high thermoelectric figure of merit (zT). However, the translation of material properties to device performance has limited success. Here, we demonstrate single-filling n-type Yb0.25Fe0.25Co3.75Sb12 and multi-filling La0.7Ti0.1Ga0.1Fe2.7Co1.3Sb12 skutterudites with a maximum zT of ~1.3 at 740 K and ~0.97 at 760 K. The peak zT of skutterudites usually occurs above 800 K, but, as shown here, the shift in peak zT to lower temperatures is beneficial for enhancing conversion efficiency at a lower hot-side temperature. In this work, we have demonstrated that the Fe-substitution significantly reduces the thermal conductivity of n-type skutterudite, closer to p-type skutterudite thermal conductivity, resulting in a module that is more compatible to operate at elevated temperatures. A uni-couple skutterudite module was fabricated using a molybdenum electrode and Ga–Sn liquid metal as the thermal interface material. A conversion efficiency of 7.27% at a low temperature gradient of 366 K was achieved, which is among the highest efficiencies reported in the literature at this temperature gradient. These results highlight that peak zT shift and optimized module design can improve conversion efficiency of thermoelectric modules at a low temperature gradient.
- Optical properties of Pb0.52Zr0.48TiO3 nanorod arrays: second harmonic generation and multiphoton carrier dynamicsMudiyanselage, Rathsara R. H. H.; Burton, John; Magill, Brenden A.; McMillan, Kiara; Gagliano, Gabriella; Morral, Ada J.; Kang, Min Gyu; Kang, Han Byul; Priya, Shashank; Stanton, Christopher J.; Khodaparast, Giti A. (2021-07)Nonlinear optical properties of poled and unpoled, lead zirconate-titanate (Pb0.52Zr0.48TiO3) nanorod arrays, grown on Pt-coated Si with similar to 200 nm diameter and similar to 600 nm height, were investigated. Clear signatures of second harmonic generations (SHG), from 490-525 nm (2.38-2.53 eV) at room temperature, were observed. Furthermore, time resolved differential reflectivity measurements were performed to study dynamical properties of photoexcited carriers in the range of 690-1000 nm where multiphoton processes were responsible for the photo-excitations. We compared this excitation scheme, which is sensitive mainly to the surface states, to when the photoexcited energy (similar to 3.1 eV) was close to the band gap of the nanorods. Our results offer promises for employing these nanostructures in nonlinear photonic applications.
- Room temperature ferromagnetic resonance in hetero-epitaxial BTO-BFO/LSMO magnetoelectric compositeMadon, Benjamin; Kang, Han Byul; Kang, Min-Gyu; Maurya, Deepam; Magill, Brenden A.; Alves, Marcos J.P.; Wegrowe, Jean-Eric; Drouhin, Henri-Jean; Priya, Shashank; Khodaparast, Giti A. (American Institute of Physics, 2018-10-30)We synthesized epitaxial BTO-BFO heterostructure with decreased leakage and simultaneously improved the multiferroic properties. This study provides new direction for ferromagnetic resonance studies, in high quality BTO-BFO films grown on LSMO. We observed small Gilbert damping (=0.004) and the absence of large inhomogeneous broadening, in a film with 80 nm thickness of BTO-BFO on LSMO (110). This fact offers opportunities for employing this material system for spin transfer in multifunctional materials where controlling magnetization by a flow of spin angular momentum, or spin current, is crucial toward developing nanoscale spin-based memory and devices. Magnetic insulators, such as BTO-BFO on LSMO, are potentially excellent candidates for pure spin current without the existence of charge current.
- Thermo-Magneto-Electric Generator Arrays for Active Heat Recovery SystemChun, Jinsung; Song, Hyun-Cheol; Kang, Min-Gyu; Kang, Han Byul; Kishore, Ravi Anant; Priya, Shashank (Springer Nature, 2017-02-01)Continued emphasis on development of thermal cooling systems is being placed that can cycle low grade heat. Examples include solar powered unmanned aerial vehicles (UAVs) and data storage servers. The power efficiency of solar module degrades at elevated temperature, thereby, necessitating the need for heat extraction system. Similarly, data centres in wireless computing system are facing increasing efficiency challenges due to high power consumption associated with managing the waste heat. We provide breakthrough in addressing these problems by developing thermo-magneto-electric generator (TMEG) arrays, composed of soft magnet and piezoelectric polyvinylidene difluoride (PVDF) cantilever. TMEG can serve dual role of extracting the waste heat and converting it into useable electricity. Near room temperature second-order magnetic phase transition in soft magnetic material, gadolinium, was employed to obtain mechanical vibrations on the PVDF cantilever under small thermal gradient. TMEGs were shown to achieve high vibration frequency at small temperature gradients, thereby, demonstrating effective heat transfer.