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Direct electrochemical synthesis of oxygenates from ethane using phosphate-based electrolysis cells

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dc.contributor.authorHonda, Yusukeen
dc.contributor.authorFujiwara, Naoyaen
dc.contributor.authorTada, Shoheien
dc.contributor.authorKobayashi, Yasukazuen
dc.contributor.authorOyama, Shigeo Teden
dc.contributor.authorKikuchi, Ryujien
dc.contributor.departmentChemical Engineeringen
dc.date.accessioned2020-12-07T19:34:46Zen
dc.date.available2020-12-07T19:34:46Zen
dc.date.issued2020-09-28en
dc.description.abstractEthane was converted directly to acetaldehyde and ethanol by partial oxidation at 220 degrees C and ambient pressure using an electrolysis cell with a proton-conducting electrolyte, CsH2PO4/SiP2O7, and Pt/C electrodes. The ethane conversion and the selectivity to the products increased with the voltage applied to the cell. It was found that O species generated by water electrolysis functioned as a favorable oxidant for partial oxidation of ethane on the Pt/C anode at intermediate temperatures. The production rates of acetaldehyde and ethanol recorded in this study were significantly higher than those in preceding reports.en
dc.format.mimetypeapplication/pdfen
dc.identifier.doihttps://doi.org/10.1039/d0cc05111jen
dc.identifier.eissn1364-548Xen
dc.identifier.issn1359-7345en
dc.identifier.issue76en
dc.identifier.pmid32902545en
dc.identifier.urihttp://hdl.handle.net/10919/101034en
dc.identifier.volume56en
dc.language.isoenen
dc.rightsCreative Commons Attribution-NonCommercial 4.0 Internationalen
dc.rights.urihttp://creativecommons.org/licenses/by-nc/4.0/en
dc.titleDirect electrochemical synthesis of oxygenates from ethane using phosphate-based electrolysis cellsen
dc.title.serialChemical Communicationsen
dc.typeArticle - Refereeden
dc.type.dcmitypeTexten
dc.type.dcmitypeStillImageen

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