Efficacy of corrosion control and pipe replacement in reducing citywide lead exposure during the Flint, MI water system recovery

dc.contributor.authorRoy, Siddharthaen
dc.contributor.authorEdwards, Marc A.en
dc.contributor.departmentCivil and Environmental Engineeringen
dc.date.accessioned2020-08-25T18:36:54Zen
dc.date.available2020-08-25T18:36:54Zen
dc.date.issued2020-08-25en
dc.description.abstractFlint biosolids monitoring data demonstrate a sustained decline in total lead release to potable water from plumbing since the 2014–2015 Flint Water Crisis (FWC), due to enhanced corrosion control treatment (3 mg L−1 orthophosphate as PO4) and removing of ∼80% of lead and galvanized iron service lines through early 2020. The official 90th percentile water lead levels, which have now met the federal Lead and Copper Rule threshold of 15 μg L−1 for the last four years, are in agreement with those predicted by a previously established biosolids regression model. There is also no longer a correlation between the percentage of children under 6 years of age with blood lead ≥ 5 μg dL−1 and biosolids lead mass in the 44 months post-FWC (Nov 2015–Jun 2019), nor are there continued correlations between plumbing-related metals in the biosolids, with the exception of Cu:Zn found in brass alloys that remain installed in homes. After Flint achieves 100% replacement of lead and galvanized service line pipes, a biosolids data analysis predicts that the remaining sources of waterborne lead including leaded brass, lead solder and legacy lead in pipe scale, will still release about 16–28% of the pre-FWC lead mass to potable water. The efficacy of enhanced corrosion control and replacement of service lines that contain lead is, therefore, on the order of 72–84% effective at reducing citywide lead exposure, yet some significant water lead sources will still remain even after pipe replacement is complete.en
dc.format.mimetypeapplication/pdfen
dc.identifier.doihttps://doi.org/10.1039/D0EW00583Een
dc.identifier.urihttp://hdl.handle.net/10919/99846en
dc.language.isoenen
dc.publisherRoyal Society of Chemistryen
dc.rightsCreative Commons Attribution-NonCommercial 4.0 Internationalen
dc.rights.urihttp://creativecommons.org/licenses/by-nc/4.0/en
dc.titleEfficacy of corrosion control and pipe replacement in reducing citywide lead exposure during the Flint, MI water system recoveryen
dc.title.serialEnvironmental Science: Water Research & Technologyen
dc.typeArticle - Refereeden
dc.type.dcmitypeTexten

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