Spatial and Temporal Analysis of Sodium-Ion Batteries

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dc.contributor.authorHou, Dewenen
dc.contributor.authorXia, Daweien
dc.contributor.authorGabriel, Ericen
dc.contributor.authorRussell, Joshua A.en
dc.contributor.authorGraff, Kincaiden
dc.contributor.authorRen, Yangen
dc.contributor.authorSun, Cheng-Junen
dc.contributor.authorLin, Fengen
dc.contributor.authorLiu, Yuzien
dc.contributor.authorXiong, Huien
dc.date.accessioned2022-09-14T14:31:42Zen
dc.date.available2022-09-14T14:31:42Zen
dc.date.issued2021-11-12en
dc.description.abstractAs a promising alternative to the market-leading lithiumion batteries, low-cost sodium-ion batteries (SIBs) are attractive for applications such as large-scale electrical energy storage systems. The energy density, cycling life, and rate performance of SIBs are fundamentally dependent on dynamic physiochemical reactions, structural change, and morphological evolution. Therefore, it is essential to holistically understand SIBs reaction processes, degradation mechanisms, and thermal/mechanical behaviors in complex working environments. The recent developments of advanced in situ and operando characterization enable the establishment of the structure-processing-property- performance relationship in SIBs under operating conditions. This Review summarizes significant recent progress in SIBs exploiting in situ and operando techniques based on X-ray and electron analyses at different time and length scales. Through the combination of spectroscopy, imaging, and diffraction, local and global changes in SIBs can be elucidated for improving materials design. The fundamental principles and state-of-the-art capabilities of different techniques are presented, followed by elaborative discussions of major challenges and perspectives.en
dc.description.notesD.H., E.G., J.R., K.G., Y.L., and H.X. acknowledge the funding support by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences program under Award Number DE-SC0019121. The work at Virginia Tech was supported by the National Science Foundation under no. CBET 1912885 and the USDA AFRI Foundational and Applied Program (grant number 2020-67021-31139). Use of the Center for Nanoscale Materials, an Office of Science user facility, was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. This research used resources of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, and was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357, and the Canadian Light Source, and its funding partners.en
dc.description.sponsorshipU.S. Department of Energy, Office of Science, Office of Basic Energy Sciences program [DE-SC0019121]; National Science Foundation [CBET 1912885]; USDA AFRI Foundational and Applied Program [2020-67021-31139]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; U.S. DOE [DE-AC02-06CH11357]; Canadian Light Sourceen
dc.description.versionPublished versionen
dc.format.mimetypeapplication/pdfen
dc.identifier.doihttps://doi.org/10.1021/acsenergylett.1c01868en
dc.identifier.issn2380-8195en
dc.identifier.issue11en
dc.identifier.pmid34805527en
dc.identifier.urihttp://hdl.handle.net/10919/111827en
dc.identifier.volume6en
dc.language.isoenen
dc.publisherAmerican Chemical Societyen
dc.rightsCreative Commons Attribution-NonCommercial-NoDerivatives 4.0 Internationalen
dc.rights.urihttp://creativecommons.org/licenses/by-nc-nd/4.0/en
dc.subjecttransmission electron-microscopyen
dc.subjectin-situ temen
dc.subjectx-ray-diffractionen
dc.subjectpair distribution functionen
dc.subjecthigh-capacity anodeen
dc.subjectoxide conversion electrodesen
dc.subjectanionic redox activityen
dc.subjectcathode materialen
dc.subjectlithium-ionen
dc.subjectelectrochemical sodiationen
dc.titleSpatial and Temporal Analysis of Sodium-Ion Batteriesen
dc.title.serialACS Energy Lettersen
dc.typeArticle - Refereeden
dc.type.dcmitypeTexten

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