2D Hierarchical Microbarcodes with Expanded Storage Capacity for Optical Multiplex and Information Encryption

dc.contributor.authorWorch, Joshen
dc.contributor.authorXie, Yujieen
dc.contributor.authorTong, Zaizaien
dc.contributor.authorRho, Juliaen
dc.contributor.authorDove, Andrewen
dc.contributor.authorO'Reilly, Rachelen
dc.date.accessioned2024-02-19T19:55:39Zen
dc.date.available2024-02-19T19:55:39Zen
dc.date.issued2023-11-28en
dc.description.abstractThe design of nanosegregated fluorescent tags/barcodes by geometrical patterning with precise dimensions and hierarchies could integrate multilevel optical information within one carrier and enhance microsized barcoding techniques for ultrahigh-density optical data storage and encryption. However, precise control of the spatial distribution in micro/nanosized matrices intrinsically limits the accessible barcoding applications in terms of material design and construction. Here, crystallization forces are leveraged to enable a rapid, programmable molecular packing and rapid epitaxial growth of fluorescent units in 2D via crystallization-driven self-assembly. The fluorescence encoding density, scalability, information storage capacity, and decoding techniques of the robust 2D polymeric barcoding platform are explored systematically. These results provide both a theoretical and an experimental foundation for expanding the fluorescence storage capacity, which is a longstanding challenge in state-of-the-art microbarcoding techniques and establish a generalized and adaptable coding platform for high-throughput analysis and optical multiplexing.en
dc.description.versionPublished versionen
dc.format.mimetypeapplication/pdfen
dc.identifier.doihttps://doi.org/10.1002/adma.202308154en
dc.identifier.orcidWorch, Joshua [0000-0002-4354-8303]en
dc.identifier.urihttps://hdl.handle.net/10919/118042en
dc.language.isoenen
dc.rightsCreative Commons Attribution 4.0 Internationalen
dc.rights.urihttp://creativecommons.org/licenses/by/4.0/en
dc.title2D Hierarchical Microbarcodes with Expanded Storage Capacity for Optical Multiplex and Information Encryptionen
dc.title.serialAdvanced Materialsen
dc.typeArticle - Refereeden
dc.type.dcmitypeTexten
dc.type.otherArticleen
pubs.organisational-group/Virginia Techen
pubs.organisational-group/Virginia Tech/Scienceen
pubs.organisational-group/Virginia Tech/Science/Chemistryen
pubs.organisational-group/Virginia Tech/All T&R Facultyen
pubs.organisational-group/Virginia Tech/Science/COS T&R Facultyen

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